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Increased Fluorescence of PbS Quantum Dots in Photonic Crystals by Excitation Enhancement

机译:光子晶体中pbs量子点的荧光增强   激励增强

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摘要

We report on enhanced fluorescence of lead sulfide quantum dots interactingwith leaky modes of slab-type silicon photonic crystals. The photonic crystalslabs were fabricated supporting leaky modes in the near infrared wavelengthrange. Lead sulfite quantum dots which are resonant the same spectral rangewere prepared in a thin layer above the slab. We selectively excited the leakymodes by tuning wavelength and angle of incidence of the laser source andmeasured distinct resonances of enhanced fluorescence. By an appropriateexperiment design, we ruled out directional light extraction effects anddetermined the impact of enhanced excitation. Three-dimensional numericalsimulations consistently explain the experimental findings by strong near-fieldenhancements in the vicinity of the photonic crystal surface. Our studyprovides a basis for systematic tailoring of photonic crystals used inbiological applications such as biosensing and single molecule detection, aswell as quantum dot solar cells and spectral conversion applications.
机译:我们报告了与平板型硅光子晶体的泄漏模式相互作用的硫化铅量子点增强的荧光。所制造的光子晶体平板在近红外波长范围内支持泄漏模式。在平板上方的薄层中制备了共振相同光谱范围的亚硫酸铅量子点。我们通过调节激光源的波长和入射角并测量增强荧光的不同共振选择性地激发了泄漏模式。通过适当的实验设计,我们排除了定向光提取的影响,并确定了增强激发的影响。三维数值模拟通过光子晶体表面附近的强近场增强一致地解释了实验结果。我们的研究为用于生物应用(例如生物传感和单分子检测)以及量子点太阳能电池和光谱转换应用的光子晶体进行系统的剪裁提供了基础。

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